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- W2003016049 abstract "Fragmentations of tautomers of the α-centered radical triglycine radical cation, [GGG•]+, [GG•G]+, and [G•GG]+, are charge-driven, giving b-type ions; these are processes that are facilitated by a mobile proton, as in the fragmentation of protonated triglycine (Rodriquez, C. F. et al. J. Am. Chem. Soc. 2001, 123, 3006–3012). By contrast, radical centers are less mobile. Two mechanisms have been examined theoretically utilizing density functional theory and Rice-Ramsperger-Kassel-Marcus modeling: (1) a direct hydrogen-atom migration between two α-carbons, and (2) a two-step proton migration involving canonical [GGG]•+ as an intermediate. Predictions employing the latter mechanism are in good agreement with results of recent CID experiments (Chu, I. K. et al. J. Am. Chem. Soc. 2008, 130, 7862–7872)." @default.
- W2003016049 created "2016-06-24" @default.
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- W2003016049 date "2009-06-01" @default.
- W2003016049 modified "2023-10-02" @default.
- W2003016049 title "Kinetics for tautomerizations and dissociations of triglycine radical cations" @default.
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- W2003016049 doi "https://doi.org/10.1016/j.jasms.2009.01.014" @default.
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