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• W2003088529 abstract "The transition from isolated and finite oxygen vacancy clusters in disordered cubic perovskites to structures containing infinite chains of oxygen vacancies in an ordered arrangement was investigated by a combined Mossbauer spectroscopy, X-ray and electron diffraction and high-resolution transmission electron microscopic study. With increasing defect concentration (equivalent to an increase in the CaFeO2.5 component concentration) and/or decreasing annealing temperature, a disorder–order phase transition occurs leading to infinite chains of vacancies in the [101]cubic direction, arranged in sheets containing essentially tetrahedral iron. In the early stages of the ordering process and at low iron concentrations, these sheets exhibit orientational disorder with two different directions of vacancy chains in addition to stacking disorder with variable sequences of tetrahedral and octahedral layers. At higher vacancy concentrations, ordered layer sequences with proportions defined by stoichiometry are formed. The ordering of vacancies into infinite chains and sheets leads to a large and discontinuous decrease in ionic conductivity." @default.
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• W2003088529 date "2000-01-01" @default.
• W2003088529 modified "2023-09-24" @default.
• W2003088529 title "The transition from short-range to long-range ordering of oxygen vacancies in CaFexTi1-xO3-x/2 perovskites" @default.
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• W2003088529 doi "https://doi.org/10.1039/b003847o" @default.
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