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- W2003155377 abstract "Abstract By describing the bimolecular kinetics a multiparticle problem is solved. The state of the system is described not by the mean number of particles (or concentration), but by the set of probabilities PN(t), N=0, 1, 2, …, N0, that the system consists of N particles. This is especially important for systems comprised of a small number of particles grouped into clusters or spurs. The probabilities PN(t) are interrelated by balance equations. The rates of transfer of the system between states with different N depend on the spatial distribution of particles and are calculated in a biparticle approximation. The theoretical results are compared with a Monte Carlo simulation of the kinetics. The fluctuational asymptote of bimolecular kinetics at long times is also discussed." @default.
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- W2003155377 date "1988-05-01" @default.
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- W2003155377 title "Diffusion-controlled kinetics of systems containing a finite number of reacting particles" @default.
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- W2003155377 doi "https://doi.org/10.1016/0301-0104(88)87022-8" @default.
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