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Matches in SemOpenAlex for { <https://semopenalex.org/work/W2003160909> ?p ?o ?g. }

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• W2003160909 abstract "A series of copper(I)−α-ketocarboxylate complexes have been prepared and shown to exhibit variable coordination modes of the α-ketocarboxylate ligand. Reaction with O2 induces decarboxylation of this ligand, and the derived copper−oxygen intermediate(s) has been intercepted, resulting in hydroxylation of an arene substituent on the supporting N-donor ligand. Theoretical calculations have provided intriguing mechanistic notions for the process, notably implicating hydroxylation pathways that involve novel [CuI−OOC(O)R] and [CuII−O-• ↔ CuIIIO2-]+ species." @default.
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• W2003160909 date "2007-10-25" @default.
• W2003160909 modified "2023-10-16" @default.
• W2003160909 title "Copper(I)−α-Ketocarboxylate Complexes: Characterization and O₂ Reactions That Yield Copper−Oxygen Intermediates Capable of Hydroxylating Arenes" @default.
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• W2003160909 doi "https://doi.org/10.1021/ja0760426" @default.
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