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- W2003173612 abstract "Hydrogen chemisorption on graphene receptor-substrate is of great interest for energy storage. However, it is difficult to reconcile with a single H atom binding to carbon being weaker than it is within initial molecular ${text{H}}_{2}$. This paradox is resolved by presenting the process as phase nucleation in the reaction ${text{Rec}}^{text{solid}}+{text{H}}_{2}^{text{gas}}ensuremath{leftrightarrow}{(text{H}ensuremath{cdot}text{Rec})}^{text{solid}}$, with the nucleus' energy separable into the Gibbs formation potential and the interface part. Atomistic calculations bridge remarkably with the macroscopic-continuum description and show a feasible path to $7.7text{ }text{wt}text{ }%$ H content at nearly ambient conditions." @default.
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- W2003173612 date "2008-07-14" @default.
- W2003173612 modified "2023-10-16" @default.
- W2003173612 title "Hydrogen storage by spillover on graphene as a phase nucleation process" @default.
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- W2003173612 doi "https://doi.org/10.1103/physrevb.78.041402" @default.
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