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- W2003200890 abstract "We evaluate the effects of lithium salt on the charge–discharge performance of a graphite negative electrode in 1-ethyl-3-methylimidazolium bis(fluorosulfonyl)imide (EMImFSI) ionic liquid-based electrolytes. Although the graphite negative electrode exhibits good cyclability and rate capability in both 0.43 mol dm−3 LiFSI/EMImFSI and LiTFSI/EMImFSI (TFSI− = bis(trifluoromethylsulfonyl)imide) at room temperature, only the LiFSI/EMImFSI system enables the graphite electrode to be operated with sufficient discharge capacity at the low temperature of 0 °C, even though there is no noticeable difference in ionic conductivity, compared with LiTFSI/EMImFSI. Furthermore, a clear difference in the low-temperature behaviors of the two cells composed of EMImFSI with a high-concentration of lithium salts is observed. Additionally, charge–discharge operation of the graphite electrode at C-rate of over 5.0 can be achieved using of the high-concentration LiFSI/EMImFSI electrolyte. Considering the low-temperature characteristics in both high-concentration electrolytes, the stable and rapid charge–discharge operation in the high-concentration LiFSI/EMImFSI is presumably attributed to a suitable electrode/electrolyte interface with low resistivity. These results suggest that optimization of the electrolyte composition can realize safe and high-performance lithium-ion batteries that utilize ionic liquid-based electrolytes." @default.
- W2003200890 created "2016-06-24" @default.
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- W2003200890 date "2015-04-01" @default.
- W2003200890 modified "2023-10-02" @default.
- W2003200890 title "Design of an electrolyte composition for stable and rapid charging–discharging of a graphite negative electrode in a bis(fluorosulfonyl)imide-based ionic liquid" @default.
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- W2003200890 doi "https://doi.org/10.1016/j.jpowsour.2015.01.070" @default.
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