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• W2003344512 abstract "The adsorption of molecules on rare-earth (0001) thin films on W(110) at room temperature has been studied using photoemission spectroscopy. ${mathrm{CO}}_{2}$ adsorbs dissociatively, up to monolayer coverage, forming a carbonate species, with clean up of adventitious hydrogen also observed. Higher coverages result in molecular adsorption. ${mathrm{H}}_{2}mathrm{O}$ and ${mathrm{H}}_{2}mathrm{S}$ on Y(0001) also adsorb dissociatively, resulting in atomic H and S, up to monolayer coverage. Higher coverages of ${mathrm{H}}_{2}mathrm{O}$ result in oxidation of the substrate to ${mathrm{Y}}_{2}{mathrm{O}}_{3},$ with formation of ${mathrm{H}}_{2}mathrm{O}$ multilayers. ${mathrm{H}}_{2}mathrm{S}$ dissociation appears to result in atomic S, adsorbed in both hollow and bridge sites. No indication of ${mathrm{CH}}_{4}$ adsorption was seen on Y(0001). These results, and those from the literature, are compared to data from bulk single-crystal rare-earth (0001) surfaces in an attempt to explain the origin of certain unexplained photoemission features observed on those surfaces." @default.
• W2003344512 created "2016-06-24" @default.
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• W2003344512 date "2003-11-05" @default.
• W2003344512 modified "2023-10-16" @default.
• W2003344512 title "Molecular adsorption on the (0001) surfaces of rare-earth metals" @default.
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• W2003344512 doi "https://doi.org/10.1103/physrevb.68.205404" @default.
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