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• W2003466775 abstract "Anelastic relaxation experiments on Sc3+-doped ceria were undertaken in order to better understand the origin of the very high Sc-V0 association energy obtained from conductivity data (where V0 = oxygen vacancy). Instead of a simple anelastic peak due to the relaxation of pairs, as found for Y3+-doped ceria, a broad peak (made up of at least 2 Debye peaks) was found in the range of activation enthalpy Hr = 0.45 to 0.54 eV. Unexpectedly, an additional small peak was observed at lower temperatures, for which Hr = 0.21 eV. The dependence of this peak on double doping (i.e. with both Sc3+ and Y3+) suggests that it is due to Sc'Ce defects, which would have to go off-center in order to account for the relaxation. Computer simulation calculations have demonstrated a modified off-center behavior in which nn O2- ions are displaced asymmetrically to a stable dipolar configuration." @default.
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• W2003466775 date "1983-12-01" @default.
• W2003466775 modified "2023-10-17" @default.
• W2003466775 title "Study of Sc2O3-doped ceria by anelastic relaxation" @default.
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• W2003466775 doi "https://doi.org/10.1016/0167-2738(83)90113-3" @default.
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