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- W2003540551 abstract "Highly loaded Co/SiO2 catalysts were prepared by a co-precipitation technique with an n-butanol drying process for Fischer–Tropsch synthesis (FTS). With the increase in cobalt loading from 20% to 80%, the FTS activity of the catalysts increased greatly. The addition of ZrO2 improved the dispersion of cobalt and promoted the adsorption of H2 and CO on cobalt. The preadsorbed H atoms significantly enhanced the adsorption of CO and C2H4, especially on cobalt promoted by ZrO2. While the adsorption of C2H4 onto clean cobalt led to the formation of ethylidyne, π- and di-σ-bonded C2H4 might form on the CO-preadsorbed 80%Co/SiO2 and 80%Co–8%ZrO2/SiO2, respectively. The presence of ZrO2 strengthened the bonding of molecularly adsorbed ethylene and increased its uptake on CO-preadsorbed cobalt, which might be why the 80%Co–8%ZrO2/SiO2 exhibited such high activity for the hydrogenation of CO to heavy hydrocarbons." @default.
- W2003540551 created "2016-06-24" @default.
- W2003540551 creator A5022585131 @default.
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- W2003540551 date "2011-04-01" @default.
- W2003540551 modified "2023-10-17" @default.
- W2003540551 title "Microcalorimetric adsorption studies of highly loaded Co–ZrO2/SiO2 catalysts for Fischer–Tropsch synthesis" @default.
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- W2003540551 doi "https://doi.org/10.1016/j.jcat.2011.01.014" @default.
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