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- W2003672064 abstract "A spike peak superimposed on the oxygen reduction wave, which usually is not evident under atmospheric conditions, was observed on gold electrodes in both and eutectic melts under pressurized conditions. It has been analyzed by cyclic voltammetry as a function of carbonate composition, total oxidant gas pressure, oxidant gas composition and cathode electrode material. The spike peak appears distinctly in melts, because its peak potential in is located 30 mV more negative than in . The charge represented by the spike peak was found to be about 5.1 μC/cm2, corresponding to less than a monolayer quantity (θ ∼ 1/100). The spike current was proportional to the scan rate, indicating a surface redox reaction associated with the oxygen reduction process. Considering the electron‐transfer mechanism of oxygen reduction, we discuss this phenomenon as an electrochemical adsorption/desorption step of an intermediate oxygen species adsorbed on a bare gold surface." @default.
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- W2003672064 date "1996-07-01" @default.
- W2003672064 modified "2023-09-26" @default.
- W2003672064 title "A Kinetic Study of Spike Peaks Observed under Pressurized Oxidant Gas Atmospheres in Molten Alkali Carbonates" @default.
- W2003672064 doi "https://doi.org/10.1149/1.1836999" @default.
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