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• W2003805231 abstract "Vibrational predissociation spectroscopy of protonated methanol clusters (tetramers and pentamers) reveals linear and cyclic structural isomers in a supersonic expansion. The cyclic pentamer, containing a five-membered ring, is identified by its characteristic free-OH stretch at 3647 cm-1 and hydrogen-bonded OH stretches at 3448 and 3461 cm-1. Ab initio calculations indicate that the excess proton in these clusters can be either localized on one methanol unit in cyclic CH3OH2+(CH3OH)3 and linear CH3OH2+(CH3OH)4 or delocalized between two methanol molecules in linear C2H9O2+(CH3OH)2 and cyclic C2H9O2+(CH3OH)3. Dynamic intracluster proton transfer can occur upon repeated ring opening and closing. The association of this process with the anomalously high proton mobility in liquid methanol is discussed." @default.
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• W2003805231 date "1999-04-01" @default.
• W2003805231 modified "2023-09-24" @default.
• W2003805231 title "Isomeric Transitions between Linear and Cyclic H⁺(CH₃OH)_4,5: Implications for Proton Migration in Liquid Methanol" @default.
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• W2003805231 doi "https://doi.org/10.1021/jp983871s" @default.
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