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- W2003863867 abstract "A theoretical framework for the description of the pulse-induced reaction dynamics of molecules interacting with short, intense laser pulses is derived. Born–Oppenheimer adiabaticity is formulated in terms of quasistationary Floquet states; its violation and the structure of the potential mixing electronic levels, and thus effecting this violation, is discussed; it is shown that, on the basis of quasistationary states, this potential is (to a very good approximation) nonvanishing only around near degeneracies in the quasienergy spectrum where it has a simple two-level structure. Ab initio calculations showing the effectivity of this scheme are performed for the H2 molecule. Particular emphasis is put on bond-softening reactions; a new mechanism is described." @default.
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- W2003863867 date "1996-06-08" @default.
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- W2003863867 title "Molecules interacting with short, intense laser pulses: The dynamical role of quasistationary states" @default.
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- W2003863867 doi "https://doi.org/10.1063/1.471628" @default.
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