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• W2004015965 abstract "Abstract. Atmospheric aerosol particles influence global climate as well as impair air quality through their effects on atmospheric visibility and human health. Ultrafine (<100 nm) particles often dominate aerosol numbers, and nucleation of atmospheric vapors is an important source of these particles. To have climatic relevance, however, the freshly-nucleated particles need to grow in size. We combine observations from two continental sites (Egbert, Canada and Hyytiälä, Finland) to show that condensation of organic vapors is a crucial factor governing the lifetimes and climatic importance of the smallest atmospheric particles. We demonstrate that state-of-the-science organic gas-particle partitioning models fail to reproduce the observations, and propose a modeling approach that is consistent with the measurements. We demonstrate the large sensitivity of climatic forcing of atmospheric aerosols to these interactions between organic vapors and the smallest atmospheric nanoparticles – highlighting the need for representing this process in global climate models." @default.
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• W2004015965 date "2011-01-06" @default.
• W2004015965 modified "2023-10-01" @default.
• W2004015965 title "Organic condensation – a vital link connecting aerosol formation to climate forcing" @default.
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• W2004015965 doi "https://doi.org/10.5194/acpd-11-387-2011" @default.
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