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- W2004039359 abstract "The sulfuric acid anion (HSO4- or SO42-) adsorbed on Pd single-crystal electrodes was studied using infrared reflection absorption spectroscopy (IRAS) in 0.05 M H2SO4 solution. Surfaces examined are flat ones (Pd(111) and Pd(100)) and stepped ones (Pd(110) (= 2(111)−(111)) and Pd(311) (= 2(111)−(100))). All of the surfaces give a single IRAS band around 1200 cm-1 that is assigned to S−O stretching vibration. The integrated band intensity depends on the crystal orientation significantly, i.e., Pd(311) ∼ Pd(110) ≪ Pd(100) < Pd(111), showing that the flat surfaces adsorb more sulfuric acid anion than the stepped ones. Magnitude of the band shift (dν/dE) on the flat surfaces is nearly twice as high as that on the stepped ones." @default.
- W2004039359 created "2016-06-24" @default.
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- W2004039359 date "2002-08-10" @default.
- W2004039359 modified "2023-09-29" @default.
- W2004039359 title "Infrared Reflection Absorption Spectroscopy of the Sulfuric Acid Anion on Low and High Index Planes of Palladium" @default.
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- W2004039359 doi "https://doi.org/10.1021/jp020898+" @default.
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