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• W2004166208 abstract "Considerable quantities, > 3 monolayers, of hydrogen (deuterium) were absorbed in subsurface sites at Ni(100) surfaces via impact of thermal H (D) atoms. Competitive to a direct transition (penetration) into the bulk with an initial probability of 4.5 × 10−2 impinging H (D) atoms abstract adsorbed D (H) with an initial abstraction probability R = 0.25 and cross section of 1.6 Å2. The filling of subsurface sites obeys a Langmuir-type rate law. An adsorbed H (D) monolayer does not affect the probability for penetration into the bulk. Above 150 K subsurface H (D) move to the surface and either recombine with adsorbed H (D) followed by recombinative desorption or get adsorbed at the surface if they encounter an empty site. The desorption kinetics from subsurface sites is in quantitative agreement with thermodynamic bulk NiH data. Isotope effects were neither observed for bulk penetration nor for abstraction." @default.
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• W2004166208 date "1995-09-01" @default.
• W2004166208 modified "2023-09-24" @default.
• W2004166208 title "Interaction of thermal H atoms with Ni(100)H surfaces: through surface penetration and adsorbed hydrogen abstraction" @default.
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• W2004166208 doi "https://doi.org/10.1016/0039-6028(95)00584-6" @default.
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