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- W2004249218 abstract "Various 12-membered ring pore zeolites were employed for the reforming of “synthetic” hydrocarbon mixtures which simulate industrial naphthas. All the zeolites were dealuminated to various extents. It was found that, under the present conditions over the samples which are slightly dealuminated, bimolecular-condensation reactions followed by recracking are responsible for the relatively large selectivities of C4 paraffins. The monomolecular cracking (via pentacoordinated carbonium ions) of the latter hydrocarbons is responsible for the large generation of CH4 from the cracking of C4 paraffins. When the Si/Al ratio increases, the selectivity of methane passes through a steep minimum, while those of C3, C4, and C5 pass through a maximum. It was also found that the zeolite pore structure is a very important factor for the time on stream activity of zeolite-based catalysts. Zeolites with reduced aluminum content and pore structures, which do not favor the formation of coke precursors in their cavities, can lead to very promising catalysts for acid-catalyzed reactions. From our study a 12-membered ring pore zeolite, which demonstrates minimal coke deactivation, was identified." @default.
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- W2004249218 date "1996-01-01" @default.
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- W2004249218 title "Effect of the Si/Al Ratio and of the Zeolite Structure on the Performance of Dealuminated Zeolites for the Reforming of Hydrocarbon Mixtures" @default.
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- W2004249218 doi "https://doi.org/10.1021/ie9507639" @default.
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