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- W2004275192 abstract "Abstract We report the surface temperature dependence for Δv =+1 vibrational excitation of NO( v =2) due to collisions with Au(1 1 1) at two incidence energies. This is compared to previous measurements on Ag(1 1 1) and Cu(1 1 0). The standard model for electron hole pair mediated vibrational excitation predicts that all three metals will exhibit a nearly Arrhenius temperature dependence with the same effective activation energy. While scattering on Ag(1 1 1) and Cu(1 1 0) obey this prediction, our new results show that the temperature dependence is non-Arrhenius on Au(1 1 1). We suggest that the large spin–orbit interaction present for Au(1 1 1) surface states may be important for vibrational excitation." @default.
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- W2004275192 date "2002-10-01" @default.
- W2004275192 modified "2023-09-27" @default.
- W2004275192 title "Non-Arrhenius surface temperature dependence in vibrational excitation of NO on Au(111): possible evidence for the importance of surface electronic states" @default.
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- W2004275192 doi "https://doi.org/10.1016/s0009-2614(02)01313-1" @default.
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