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• W2004319768 abstract "When dilute solutions of nearly monodisperse (3−5-nm diameter) passivated metal nanoparticles are evaporated on a solid substrate (a transmission electron microscopy grid), the resulting submonolayer structures are annular ringlike arrays. We describe here a theoretical mechanism whereby the growth of holesdry areas of the solid surface which is otherwise wet by solventis conjectured to be responsible for the formation of these novel close-packed two-dimensional (2D) arrays. Each annular ring is argued to arise from the pinning of the rim of an opening hole by a sufficient number of particles. Hole nucleation in this ultrathin-film system can occur due to two independent driving forces: evaporation (volatile hole nucleation) and disjoining pressure (nonvolatile hole nucleation). The cases are first presented separately, in an appropriate analytical theory, and are subsequently treated jointly in the context of a simulation. We investigate in particular the effect of competing time scales (for hole nucleation, fluid flow, and solvent evaporation) on the average diameter of the resulting ringlike configurations." @default.
• W2004319768 created "2016-06-24" @default.
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• W2004319768 date "1998-05-09" @default.
• W2004319768 modified "2023-10-16" @default.
• W2004319768 title "Interplay between Hole Instability and Nanoparticle Array Formation in Ultrathin Liquid Films" @default.
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• W2004319768 doi "https://doi.org/10.1021/la971147f" @default.
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