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- W2004365715 abstract "Abstract The uranyl dication, [UO2]2+, is the most prevalent and most thermodynamically stable form of uranium and is a soluble and problematic environmental contaminant. It is also extraordinarily chemically robust due to the strongly covalent trans-UO2 bonding. In contrast, the pentavalent uranyl cation [UO2]+ is unstable in an aqueous environment with respect to disproportionation into tetravalent uranium species and [UO2]2+. Aside from fundamental interest, an understanding of the pentavalent [UO2]+ cation is desirable since it is important environmentally as a key intermediate in the precipitation of uranium from groundwater. In the last 2 years, the use of anaerobic coordination chemistry techniques and organometallic reagents has allowed the isolation of a few kinetically inert complexes containing the f1 [UO2]+ cation. The synthesis and characterisation of these, and the insight they give into subsequent reactivity of the trans-UO2 unit, is discussed in this review." @default.
- W2004365715 created "2016-06-24" @default.
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- W2004365715 date "2009-08-01" @default.
- W2004365715 modified "2023-10-05" @default.
- W2004365715 title "Pentavalent uranyl complexes" @default.
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- W2004365715 doi "https://doi.org/10.1016/j.ccr.2009.03.014" @default.
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