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- W2004389387 abstract "The fractionation of sulfur isotopes in the gas-phase reaction of OCS with OH was calculated by ab initio methods. The first reaction step occurs through a carbon bonded OH–OCS transition state. The activation barrier is 18.4 kJ mol−1 (CCSD(T)/aug-cc-pVDZ level plus zero-point energy) relative to the reactants. Fractionation constants are −1.4, −2.6 and −6.3‰ for 33S, 34S and 36S respectively. These results bring new insight regarding the origin of stratospheric sulfate aerosols, including the identification of characteristic isotopic fractionations in the lower and middle stratosphere." @default.
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- W2004389387 date "2008-01-01" @default.
- W2004389387 modified "2023-09-26" @default.
- W2004389387 title "Ab initio study of sulfur isotope fractionation in the reaction of OCS with OH" @default.
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- W2004389387 doi "https://doi.org/10.1016/j.cplett.2007.11.054" @default.
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