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• W2004395614 startingPage "1883" @default.
• W2004395614 abstract "The actinic (i.e., photolysis) wavelength dependence of chlorine dioxide (OClO) photochemistry in solution is investigated. Femtosecond pump–probe studies performed with 355-nm photoexcitation are presented for OClO dissolved in water and acetonitrile. Relative to earlier studies employing 400-nm photoexcitation, a decrease in primary-photoproduct geminate-recombination efficiency is observed in both solvents. This decrease in recombination efficiency is especially dramatic in acetonitrile where the recombination quantum yield is found to be only 0.08±0.04. The solvent and actinic-wavelength dependence of geminate recombination is discussed with respect to the recent theoretical work of Benjamin and co-workers [J. Chem. Phys. 116, 8930 (2002)]. Substantial increases in the optical density at 267 nm are also observed that cannot be explained by considering the increase in ClO concentration accompanying a reduction in geminate-recombination efficiency exclusively. Instead, these increases are consistent with an increase in the quantum yield for ClOO and/or Cl production suggesting that the partitioning between OClO photoproduct channels is actinic-wavelength dependent." @default.
• W2004395614 created "2016-06-24" @default.
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• W2004395614 date "2003-01-08" @default.
• W2004395614 modified "2023-10-02" @default.
• W2004395614 title "On the actinic wavelength dependence of OClO photochemistry in solution" @default.
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• W2004395614 doi "https://doi.org/10.1063/1.1531613" @default.
• W2004395614 hasPublicationYear "2003" @default.
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