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• W2004477992 abstract "The photoionization efficiency (PIE) spectra of metastable sulfur (S) atoms in the D1 and S1 states have been recorded in the 73350–84950cm−1 frequency range by using a velocity-mapped ion imaging apparatus that uses a tunable vacuum ultraviolet laser as the ionization source. The S(D1) and S(S1) atoms are produced by the 193nm photodissociation of CS2. The observed PIE spectra of S(D1) and S(S1) shows 35 autoionizing resonances with little or no contribution from direct photoionization into the S+(S3∕24)+e− ionization continuum. Velocity-mapped ion images of the S+ at the individual autoionizing Rydberg resonances are used to distinguish whether the lower state of the resonance originates from the D1, S1, or P3 states. The analysis and assignment of the Rydberg peaks revealed 22 new Rydberg states that were not previously known. The autoionization lifetimes τ of the Rydberg states are derived from the linewidths by fitting the lines with the Fano formula. Deviations from the scaling law of τ(n*)∝n*3, where n* is the effective quantum number of the Rydberg state, are observed. This observation is ascribed to perturbations by nearby triplet Rydberg states, which shorten the autoionization lifetimes of the singlet Rydberg levels." @default.
• W2004477992 created "2016-06-24" @default.
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• W2004477992 date "2008-02-25" @default.
• W2004477992 modified "2023-09-23" @default.
• W2004477992 title "Vacuum ultraviolet excitation spectroscopy of the autoionizing Rydberg states of atomic sulfur in the 73350–84950cm−1 frequency range" @default.
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• W2004477992 doi "https://doi.org/10.1063/1.2829403" @default.
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• W2004477992 hasPublicationYear "2008" @default.
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