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- W2004484377 abstract "Rate constants for the disproportionation reaction (1) OH + OH → H2O + O in the range 250–580 K have been measured by flash photolyzing H2O/N2 mixtures and monitoring the decay of OH using quantitative UV resonance spectrometry. The result k1 = (3.2 · 0.8) 10−12 exp (-242/T) cm3/molecule · s, does not correlate with existing high temperature data and confirms previously suggested non-Arrhenius behaviour for this reaction. On the basis of all available data the temperature variation of k1 over the range 250–2000 K is best represented by the empirical expression k1(T) = exp (-27.73 + 1.49 · 10−3T) cm3/molecule · s. The extent of the Arrhenius graph curvature can be reconciled by a “close-collision” model incorporating the energy variation of accessible product states." @default.
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- W2004484377 date "1981-12-01" @default.
- W2004484377 modified "2023-09-25" @default.
- W2004484377 title "Temperature Dependence of the Reaction OH + OH → H2O + O" @default.
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- W2004484377 doi "https://doi.org/10.1002/bbpc.19810851209" @default.
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