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- W2004554161 abstract "The observed asymmetric behaviour of mixing properties of AlMg liquid alloys around equiatomic composition with smaller negative value for excess free energy of mixing (GMXS = −0.15 KJ mol−1) has aroused our interest to undertake a theoretical investigation of this system. It will be proper to mention that various factors such as size difference and electronegativity difference are too small to account for the asymmetry in the above system. The existence of an intermetallic compound in the solid phase, which is manifested in the phase diagram, may be one of the factors for the anomalous behaviour of the properties of mixing. A simple statistical mechanical theory based on the complex-formation model (the complex AμBv is formed by the preferentialarrangement of A and B constituent atoms of the alloy AB; μA + vB⇌AμBv) has been used to investigate the phenomenon of compound formation in AlMg liquid alloys through the study of various thermodynamic as well as microscopic functions such as the excess free energy of mixing, heat of mixing, concentration fluctuations at the long-wavelength [SCC(0)], chemical short-range-order parameter (α1), etc. Our study, which explains the observed asymmetry almost successfully suggests that Al3Mg2 complexes exist in the liquid phase. But the tendency to form a compound is not so strong. The system exhibits almost ideal behaviour in the Mg-rich end (CMg>0.8). This ideal behaviour might be linked with the glass formation. But this aspect to the AlMg system requires investigation. The temperature dependence of energy parameters plays an important role in the mixing in AlMg liquid alloys." @default.
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- W2004554161 date "1996-02-01" @default.
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- W2004554161 title "Intermetallic associations in AlMg liquid alloys" @default.
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