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• W2004594963 abstract "Measurements of the static structure factor S(q) and the mean-squared displacement W(t) in suspensions of charged polystyrene spheres (polyballs), obtained by static and dynamic light scattering experiments, are discussed in terms of the one-component macroion fluid model. The self-diffusion properties are calculated using two approximations for the appropriate memory function, a mode-coupling approximation and an approximation based on the exact short-time behaviour of the dynamics. In both cases, the dynamic properties are entirely expressed in terms of the static structure factor. The latter is calculated within the rescaled mean-spherical approximation and is tested against Monte Carlo simulations (MC). Fitting the MC data to the experimental S(q), an estimate of the polyball charge is obtained. This value of the charge is then used in Brownian dynamics simulations for the mean-squared displacement. Detailed comparisons of the experimental and simulation data for W(t) show good agreement with the theoretical results." @default.
• W2004594963 created "2016-06-24" @default.
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• W2004594963 date "1988-12-01" @default.
• W2004594963 modified "2023-09-27" @default.
• W2004594963 title "Structure and self-diffusion in dilute suspensions of polystyrene spheres: Experiment vs. computer simulation and theory" @default.
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• W2004594963 doi "https://doi.org/10.1016/0378-4371(88)90232-4" @default.
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