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• W2004724943 abstract "The reaction kinetics of NCS radicals with several molecules was investigated for the first time, using laser-induced fluorescence spectroscopy to measure total rate constants and infrared absorption spectroscopy to probe possible reaction products. The NCS + NO reaction has a pressure-dependent total rate constant, with a low pressure (∼2 Torr) rate given by the expression kNCS + NO = (4.1 ± 1.4) × 10-15 exp[(1561 ± 116)/T] cm3 molecule-1 s-1 over the range 298−468 K. On the basis of the observed pressure dependence and product detection studies, this reaction is believed to be an association reaction, producing primarily NCSNO products. The NCS + NO2 reaction was pressure-independent, with a rate constant given by kNCS+NO2 = (7.0 ± 0.6) × 10-12 exp[(579 ± 39.4)/T] cm3 molecule-1 s-1 over the range 298−620 K. No reaction of NCS with C2H2 or O2 was detected, and upper limits of rate constants with these molecules were estimated at <1.0 × 10-14 cm3 molecule-1 s-1." @default.
• W2004724943 created "2016-06-24" @default.
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• W2004724943 creator A5058841795 @default.
• W2004724943 date "1999-11-25" @default.
• W2004724943 modified "2023-09-27" @default.
• W2004724943 title "Kinetics of the NCS Radical" @default.
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• W2004724943 doi "https://doi.org/10.1021/jp992930e" @default.
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