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• W2004771269 abstract "Laser desorption/ionization from structured surfaces has been the object of recently renewed interest. Conditions in the plume of material ablated from such surfaces may differ from those of a sample which is ablated in bulk. Since recombination and secondary ion–molecule reactions in the plume play a major role in determining the types and quantities of ions observed at the detector, these differences are analytically relevant. Desorption/ionization substrates with channels of high aspect ratio are modeled as capillary nozzles, from which free jets are emitted. A previously developed matrix-assisted laser desorption/ionization ablation/ionization model is adapted for these jets. More primary ions reach the detector when ablated from a capillary orifice, but fewer analye ions are created in secondary reactions. These differences in ion yield can persist for arrays of capillaries on the surface, depending on the ratio of their diameter to spacing." @default.
• W2004771269 created "2016-06-24" @default.
• W2004771269 creator A5066508058 @default.
• W2004771269 date "2009-04-01" @default.
• W2004771269 modified "2023-10-15" @default.
• W2004771269 title "Laser Desorption/Ablation Plumes from Capillary-Like Restricted Volumes" @default.
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• W2004771269 doi "https://doi.org/10.1255/ejms.960" @default.
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