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• W2004893140 abstract "Thermoelectric properties and phase evolution have been studied in biphasic Ti–Ni–Sn materials containing full-Heusler TiNi2Sn embedded within half-Heusler thermoelectric TiNiSn. Materials, prepared by levitation induction melting followed by annealing, were of the nominal starting composition of TiNi1+xSn, with x between 0.00 and 0.25. Phases and microstructure were determined using synchrotron X-ray diffraction and optical and electron microscopy. The full-Heusler phase is observed to be semi-coherent with the half-Heusler majority phase. Differential thermal analysis was performed to determine melting temperatures of the end-member compounds. The thermal conductivity is reduced with the introduction of a dispersed, full-Heusler phase within the half-Heusler material. This leads to an increased thermoelectric figure of merit, ZT, from 0.35 for the stoichiometric compound to 0.44 for TiNi1.15Sn. Beyond x = 0.15 ZT decreases due to a rise in thermal conductivity. Density functional theory calculations using hybrid functionals were performed to determine band alignments between the half- and full-Heusler compounds, as well as comparative energies of formation. The hybrid functional band structure of TiNiSn is presented as well." @default.
• W2004893140 created "2016-06-24" @default.
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• W2004893140 date "2014-01-28" @default.
• W2004893140 modified "2023-09-26" @default.
• W2004893140 title "Phase stability and property evolution of biphasic Ti–Ni–Sn alloys for use in thermoelectric applications" @default.
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• W2004893140 doi "https://doi.org/10.1063/1.4862955" @default.
• W2004893140 hasPublicationYear "2014" @default.
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