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• W2005037110 abstract "The transfers of hydrophilic ions between aqueous and organic phases are ubiquitous in biological and technological systems. These energetically unfavorable processes can be facilitated either by small molecules (ionophores) or by ion-transport proteins. In absence of a facilitating agent, ion-transfer reactions are assumed to be simple, one-step processes. Our experiments at the nanometer-sized interfaces between water and neat organic solvents showed that the generally accepted one-step mechanism cannot explain important features of transfer processes for a wide class of ions including metal cations, protons, and hydrophilic anions. The proposed new mechanism of ion transfer involves transient interfacial ion paring and shuttling of a hydrophilic ion across the mixed-solvent layer." @default.
• W2005037110 created "2016-06-24" @default.
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• W2005037110 date "2006-10-31" @default.
• W2005037110 modified "2023-10-18" @default.
• W2005037110 title "Shuttling Mechanism of Ion Transfer at the Interface between Two Immiscible Liquids" @default.
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• W2005037110 doi "https://doi.org/10.1021/ja0656090" @default.
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