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• W2005156768 startingPage "6688" @default.
• W2005156768 abstract "Lamellar inorganic–organic hybrids were prepared as powders and films via hydrolysis and cocondensation of tetraethoxysilane (TEOS) and a coumarin derivative containing a triethoxysilyl group. The formation of lamellar structures consisting of siloxane layers and interlayer coumarin groups with ca. 4 nm periodicities, revealed by XRD and TEM, is induced by self-assembly of the oligomeric species derived from TEOS and the derivative. The UV–vis absorption spectrum of the as-synthesized hybrid film showed an absorption maximum blue-shifted from that observed for a CHCl3 solution of the monomeric coumarin derivative, which supports the formation of a face-to-face structure of the interlayer coumarin groups. Dimerization of the coumarin groups occurred by irradiation with visible light (>310 nm). The groups in the lamellar hybrid film showed faster dimerization and the yield of dimers was higher, if compared with those in a disordered hybrid film and the neat coumarin derivative, indicating the efficient dimerization of the chromophores with a controlled arrangement. The molecular design of a coumarin derivative strongly influences the property of hybrids as well as the mesostructural formation." @default.
• W2005156768 created "2016-06-24" @default.
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• W2005156768 date "2010-01-01" @default.
• W2005156768 modified "2023-09-24" @default.
• W2005156768 title "Preparation of lamellar inorganic–organic hybrids from tetraethoxysilane and a coumarin derivative containing a triethoxysilyl group and photodimerization of the interlayer coumarin groups" @default.
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• W2005156768 doi "https://doi.org/10.1039/c0jm00407c" @default.
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