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• W2005246712 abstract "Mn-MCM-41 is found to be the most effective heterogeneous catalyst for the epoxidation of styrene with tert-butyl hydroperoxide (TBHP) among several metal ion-containing mesoporous molecular sieves including Mn-, V-, Cr-, Fe-, and Mo-MCM-41. ESR, XANES, diffuse reflectance UV–VIS, UV–Raman and XPS are used to characterize the Mn-MCM-41 synthesized by both direct hydrothermal (DHT) and template ion exchange (TIE) methods. The results suggest that Mn2+ and Mn3+ coexist in the Mn-MCM-41 samples synthesized by both methods and a large part of manganese atoms could be incorporated into the framework of MCM-41 obtained by the DHT method. The oxidation of either styrene or stilbene with TBHP as the oxidant over the Mn-MCM-41 produces corresponding epoxide as the main product; the reaction probably proceeds through a radical intermediate. The TIE catalyst shows higher activity, while the DHT catalyst gives higher TBHP efficiency for the epoxidation reactions." @default.
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• W2005246712 date "2002-09-01" @default.
• W2005246712 modified "2023-10-18" @default.
• W2005246712 title "Manganese-containing MCM-41 for epoxidation of styrene and stilbene" @default.
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• W2005246712 doi "https://doi.org/10.1016/s1381-1169(02)00323-0" @default.
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