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• W2005280201 abstract "In ZnS ${mathrm{the}}^{3}$${mathit{T}}_{1}$(F)${mathrm{ensuremath{-}}}^{3}$${mathit{T}}_{1}$(P) transition of isolated ${mathrm{Ni}}^{2+}$ causes structured near infrared absorption and emission bands. Crystals doped in the sub-ppm region exhibit exceptionally sharp lines suited to study the dependence on external fields. Here the fine structure of the perfectly cubic and one axial ${mathrm{Ni}}^{2+}$ center is studied. A secure assignment of the observed optical transitions is achieved on the basis of high-resolution absorption and emission investigations at various crystal temperatures and in magnetic fields up to 15 T. The experimental results give evidence for intermediate dynamical Jahn-Teller effects in both the $^{3}$${mathit{T}}_{1}$(F) ground and the $^{3}$${mathit{T}}_{1}$(P) excited state, which are attributed to the coupling to local ${mathit{T}}_{2}$-type modes. A detailed comparison shows good agreement between the experimental data for ZnS:Ni and those of the well understood system CdS:Ni. A Fano-type structure in the $^{3}$${mathit{T}}_{1}$(F)${mathrm{ensuremath{-}}}^{3}$${mathit{T}}_{1}$(P) absorption is explained by the coupling of a distinct local mode of the Ni center to a continuum of phonon states. Additionally, the interaction of low-frequency acoustical phonons with the Ni center is investigated. No thermal equilibrium is established in the excited $^{3}$${mathit{T}}_{1}$(P) state during its lifetime, which gives rise to hot emission lines." @default.
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• W2005280201 date "1994-12-15" @default.
• W2005280201 modified "2023-09-30" @default.
• W2005280201 title "High-resolution Zeeman spectroscopy ofNi2+in ZnS" @default.
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• W2005280201 doi "https://doi.org/10.1103/physrevb.50.17028" @default.
• W2005280201 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/9976099" @default.
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