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• W2005411946 abstract "The ν5+ν9 spectra of ethylene, C2H4, and its dimer, solvated in helium nanodroplets, have been recorded in the wavelength region near 1.6μm. The monomer transitions show homogeneous broadening of ≈0.5cm−1, which is interpreted as due to an upper state vibrational relaxation lifetime of ≈10ps. Nearly resonant vibrational energy transfer (ν5+ν9→2ν5) is proposed as the relaxation pathway. The dimer gives a single unresolved absorption feature located 4cm−1 to the red of the monomer band origin. The scaling of moments of inertia upon solvation in helium is 1.18 for the monomer and &gt;2.5 for the dimer. In terms of the adiabatic following approximation, this classifies the monomer as a fast rotor and the dimer as a slow rotor." @default.
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• W2005411946 date "2005-03-08" @default.
• W2005411946 modified "2023-10-18" @default.
• W2005411946 title "Near-infrared spectroscopy of ethylene and ethylene dimer in superfluid helium droplets" @default.
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• W2005411946 doi "https://doi.org/10.1063/1.1854630" @default.
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