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- W2005458375 abstract "Positively charged copolymer hydrogels based on N-isopropyl-acrylamide (NiPAAm) and a cationic surfactant monomer (surfmer) were functionalized upon electrostatic self-assembly of functional organic or inorganic complex counterions in the gel. As cationic surfmers 11-acryloylundecyltrimethylammonium bromide (AUT-MAB) or 11-methacryloyl-undecyltrimethylammonium bromide (MUTMAB) were used. The hydrogels were prepared from a micellar aqueous solution of the surfmer and NiPAAm either upon 60 Co-gamma irradiation, or upon chemical cross-linking using methylenebisacrylamide as cross-linker and 1 , 4 -diaminobutane as accelerator. Electrostatic self-assembly was facilitated utilizing the thermoresponsive swelling and shrinking of the hydrogel. Several examples of gel functionalization are described such as in-situ preparation of Prussian Blue and Pd° nanoparticles, and induction of fluorescent properties. The catalytic activity of the palladium-containing gel was studied by investigating the reduction of 4 -nitrophenol ( 4 -NP) with sodium borohydride as a model reaction. Fluorescent gels can be prepared upon exchange of bromide against 1-pyrenesulfonate ions in the gel." @default.
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- W2005458375 date "2010-12-01" @default.
- W2005458375 modified "2023-09-24" @default.
- W2005458375 title "Functionalization of Hydrogels Based on N -Isopropyl-acrylamide and Cationic Surfactant Monomers upon Electrostatic Self-Assembly" @default.
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- W2005458375 doi "https://doi.org/10.1002/masy.201000021" @default.
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