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- W2005578477 abstract "The model is used to simulate vertical profiles of H2S, SO2 and SO42− in the atmosphere up to about 8 km. Transformation and wet removal processes are treated as first order reactions with constant rate coefficients and the dry deposition is estimated using deposition velocity parameters. From a systematic study of the sensitivity of the model to variations in some of the key parameters and from a comparison with aircraft measurements of SO2 and SO42− over Scandinavia the following results are derived. An increase in the value of the deposition velocity in long range transport models beyond about 1cm s−1 has little effect on the estimated dry deposition. As the rate coefficient for the transformation of H2S to SO2 varies from 10 to 0.01 h−1 the scale height of H2S varies from 40 to 1400 m and that of SO2 (applicable to background air) from 1300 to 3400 m. An average value for the first 30 hours of the rate of transformation of man-made SO2 to SO42− is probably in the range 0.007 to 0.04 h−1 for European conditions. It is difficult to simulate the observed pattern of wet deposition of sulfur over northern Europe if the wet removal of SO2 is neglected." @default.
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- W2005578477 date "1978-01-01" @default.
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- W2005578477 title "Transformation and removal processes for sulfur compounds in the atmosphere as described by a one-dimensional time-dependent diffusion model" @default.
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- W2005578477 doi "https://doi.org/10.1016/0004-6981(78)90232-9" @default.
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