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• W2005694494 abstract "The diffusion of particles in concentrated lattice gases is studied by Monte Carlo methods, assuming a fcc lattice with repulsive nearest-neighbor interaction. Particular attention is paid to the influence of ordering on the diffusion properties, since the model has ordered superstructures at low temperatures $T$ near the stoichiometric concentrations $c=frac{1}{4}, frac{1}{2}, mathrm{and} frac{3}{4}$. Both the self-diffusion of tagged particles and the collective diffusion by which concentration fluctuations decay are obtained. In the ordered regions both diffusivities are rather small due to a strong decrease of the effective jump rate of the particles. The correlation factor $f(T,c)$ for self-diffusion has a pronounced non-monotonic concentration dependence for low temperatures. This is interpreted by reducing the problem near $T=0$ and the limits $censuremath{rightarrow}frac{1}{4}ensuremath{-},frac{1}{2}ensuremath{-}$ to an effective single-vacancy problem, and $censuremath{rightarrow}frac{1}{4}+,frac{1}{2}+$ to an effective single-particle problem. Other lattices are briefly discussed." @default.
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• W2005694494 date "1983-08-15" @default.
• W2005694494 modified "2023-09-26" @default.
• W2005694494 title "Diffusion in concentrated lattice gases. V. Particles with repulsive nearest-neighbor interaction on the face-centered-cubic lattice" @default.
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• W2005694494 doi "https://doi.org/10.1103/physrevb.28.1846" @default.
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