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- W2005731283 abstract "The structure evolution of network structure in clay−polymer aqueous solutions after shear thickening under shear deformation was investigated by means of small-angle neutron scattering (SANS; Rheo-SANS). Laponite (clay; C) platelet dispersions in poly(ethylene oxide) (PEO; P) aqueous solutions with various deuterious/hydrogeneous water compositions were prepared, and contrast-variation SANS experiments were carried out under flow field. The two-dimensional scattering contour patterns changed suddenly from isotropic to anisotropic patterns at the shear thickening transition point. The orientations of clay platelets and PEO chains were individually characterized by the partial structure factors, SCC(q), SCP(q), and SPP(q), which were obtained by decomposition of the SANS intensity functions. The SANS results show that PEO chains are adsorbed on clay platelets even in a flow field and are peeled off at the shear thickening transition point. Flow birefringence results suggest that the shear thickening is a corporation of clay and polymer chains, i.e., bridging of clays by PEO chains. Aging of the clay−PEO solutions leads to lowering the threshold of the critical shear rate at which shear thickening occurs." @default.
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- W2005731283 date "2010-08-16" @default.
- W2005731283 modified "2023-10-01" @default.
- W2005731283 title "Rheo-SANS Studies on Shear Thickening in Clay−Poly(ethylene oxide) Mixed Solutions" @default.
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- W2005731283 doi "https://doi.org/10.1021/ma101319j" @default.
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