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- W2005734971 abstract "Water oxidation to evolve O2 in photosynthesis is catalyzed by an enzyme whose active site contains a μ-oxo-bridged manganese core. Catalytic O2 evolution has been difficult to establish by manganese−oxo complexes in homogeneous aqueous solutions. The reaction of [(OH2)(terpy)MnIII(μ-O)2MnIV(terpy)(OH2)]3+ (terpy = 2,2‘:6‘,2‘ ‘-terpyridine) (1) with a CeIV oxidant leads to the decomposition of 1 to the permanganate ion without O2 evolution in an aqueous solution but catalytically produces O2 from water when 1 is adsorbed on clay compounds. 18O-labeling experiments showed that the oxygen atoms in O2 originate exclusively from water. Catalysis of O2 evolution requires cooperation of 2 equiv of 1 adsorbed on clay compounds." @default.
- W2005734971 created "2016-06-24" @default.
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- W2005734971 date "2004-06-11" @default.
- W2005734971 modified "2023-10-11" @default.
- W2005734971 title "Catalytic O<sub>2</sub> Evolution from Water Induced by Adsorption of [(OH<sub>2</sub>)(Terpy)Mn(μ-O)<sub>2</sub>Mn(Terpy)(OH<sub>2</sub>)]<sup>3+</sup> Complex onto Clay Compounds" @default.
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- W2005734971 doi "https://doi.org/10.1021/ja039780c" @default.
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