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• W2005767369 startingPage "7274" @default.
• W2005767369 abstract "Tailor-made water-soluble macromolecules, including a glycopolymer, obtained by living/controlled RAFT-mediated polymerization are demonstrated to react in water with diene-functionalized poly(ethylene glycol)s without pre- or post-functionalization steps or the need for a catalyst at ambient temperature. As previously observed in organic solvents, hetero-Diels–Alder (HDA) conjugations reached quantitative conversion within minutes when cyclopentadienyl moieties were involved. However, while catalysts and elevated temperatures were previously necessary for open-chain diene conjugation, additive-free HDA cycloadditions occur in water within a few hours at ambient temperature. Experimental evidence for efficient conjugations is provided via unambiguous ESI-MS, UV/vis, NMR, and SEC data." @default.
• W2005767369 created "2016-06-24" @default.
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• W2005767369 date "2012-04-20" @default.
• W2005767369 modified "2023-10-17" @default.
• W2005767369 title "(Ultra)Fast Catalyst-Free Macromolecular Conjugation in Aqueous Environment at Ambient Temperature" @default.
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• W2005767369 doi "https://doi.org/10.1021/ja301762y" @default.
• W2005767369 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/22506863" @default.
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