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- W2005862082 endingPage "2583" @default.
- W2005862082 startingPage "2576" @default.
- W2005862082 abstract "A series of well defined ABA, 3-arm star and bottle brush type copolymers, containing soft poly(n-butyl acrylate) (PBA) blocks and hard blocks of polystyrene (PS) were synthesized by atom transfer radical polymerization (ATRP). Small angle X-ray scattering was used to study the phase separation in these systems and dynamic mechanical analysis and tensile tests were performed to characterize their thermo-mechanical properties. The specific molecular architecture has a major effect on the copolymers self-organization and material properties. The linear ABA type copolymers showed micro phase separation and thermoplastic elastomer (TPE) behavior only at very high PS content. The change of molecular architecture from linear to 3-arm star type resulted in an improved phase separation at lower PS content and better thermoplastic elastomer properties. In contrast the specific brush type molecular architecture seems to prevent the micro phase separation of the PBA and PS components, resulting in amorphous bulk material with single glass transition temperature." @default.
- W2005862082 created "2016-06-24" @default.
- W2005862082 creator A5046695542 @default.
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- W2005862082 creator A5056539244 @default.
- W2005862082 creator A5064216660 @default.
- W2005862082 creator A5077106342 @default.
- W2005862082 creator A5081764848 @default.
- W2005862082 date "2011-05-01" @default.
- W2005862082 modified "2023-09-24" @default.
- W2005862082 title "Effect of chain topology on the self-organization and the mechanical properties of poly(n-butyl acrylate)-b-polystyrene block copolymers" @default.
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