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W2006273313 startingPage "12387" @default.
W2006273313 abstract "Aluminum tetracarboxyphthalocyanine adsorbed on TiO2 has been examined as a sensitizer for degradation of 4-chlorophenol (4-CP) in water under visible light irradiation (λ ≥ 450 nm). It was observed that 4-CP was mostly decomposed into CO2 and chloride ions, whereas the reaction rate was greatly influenced by several parameters. The optimum loading of the dye on TiO2 was about 1.0 wt %, nearly independent of TiO2 used. The solution pH which favored 4-CP degradation over the dye loaded TiO2 was about pH 7. An increase in 4-CP concentration below 0.27 mM resulted in increased rate of 4-CP degradation, the kinetics well fitted into the Langmuir−Hinshelwood equation. In the flow of N2, the reaction was almost completely inhibited. Experiments through EPR spin trapping, methanol quenching, and silver ions as electron acceptors revealed the involvement of superoxide, hydroxyl and dye cation radicals in the dye sensitized reaction. Evidence is well interpreted in terms of the electron transfer from the excited d..." @default.
W2006273313 created "2016-06-24" @default.
W2006273313 creator A5039803237 @default.
W2006273313 creator A5049968522 @default.
W2006273313 date "2009-06-12" @default.
W2006273313 modified "2023-09-26" @default.
W2006273313 title "Sensitization of TiO<sub>2</sub> with Aluminum Phthalocyanine: Factors Influencing the Efficiency for Chlorophenol Degradation in Water under Visible Light" @default.
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W2006273313 doi "https://doi.org/10.1021/jp9016882" @default.
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