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- W2006304462 abstract "Quantum beats in the pump−probe spectra of aqueous CdTe quantum dots were observed after the resonant excitation of phonon wavepackets with femtosecond laser pump pulses. The beats have a frequency corresponding to longitudinal optical phonon modes and are coupled to an intrinsic exciton state (1S−2S3/2). We investigated how quantum confinement influences the properties of the wavepacket motion. Our results reveal that neither the exciton−phonon coupling strength nor the optical phonon frequencies are dependent on the size of the dots. However, the observed coherence dephasing times were strongly influenced by the size of the particles. This size-dependent loss of coherence in the phonon wavepacket is correlated with the hole relaxation to the band edge of the exciton state." @default.
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- W2006304462 date "2009-02-12" @default.
- W2006304462 modified "2023-09-27" @default.
- W2006304462 title "Femtosecond Probing of Optical Phonon Dynamics in Quantum-Confined CdTe Nanocrystals" @default.
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- W2006304462 doi "https://doi.org/10.1021/jp810295m" @default.
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