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- W200640266 abstract "One of the recent trends in the development of heterogeneous catalysts is connected with metal-containing zeolites. Metal cations can be introduced into a zeolite at the synthesis stage as well as through various methods of zeolite modification. There are a number of unique catalysts showing high activity and selectivity in the diverse processes. Typical examples of such catalysts and processes are Ti-containing zeolites, Fe zeolites, Zn and Ga zeolite, and Cu, Fe, and Co zeolites. Fine dispersion of the active component seems to be one of the main factors that make molecular sieves very promising for the development of efficient catalysts. Another aspect of the correlation between the stability and reactivity of the cation species relates to possible competition between different structural forms of the cations located in various positions of the zeolite matrix. The main problem of computer modeling of structures relates to accounting the structural relaxation of the lattice in the formation of hydro-peroxide activation intermediate, as the latter process is accompanied by the hydrolysis of the lattice bonds. The formation of cationic positions of monovalent metal ions in zeolites is determined by the distribution of aluminum through zeolite lattice. Stabilization of multivalent metal ions in zeolites can be achieved by the incorporation of ELO into the structure and formation of bi- or multinuclear complexes, wherein each cation interacts efficiently only with the zeolite fragment containing a single Al ion." @default.
- W200640266 created "2016-06-24" @default.
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- W200640266 date "2004-01-01" @default.
- W200640266 modified "2023-09-26" @default.
- W200640266 title "Structure and reactivity of metal ion species in high-silica zeolites" @default.
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- W200640266 doi "https://doi.org/10.1016/b978-012164137-5/50008-x" @default.
- W200640266 hasPublicationYear "2004" @default.
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