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- W2006402753 abstract "A complete study on the energy partitioning upon laser-induced thermal desorption of aniline from silica surfaces was undertaken. The measurements include characterization of the aniline–quartz adsorption system using temperature-programmed desorption, the extrapolation of quasiequilibrium desorption temperatures to the regime of laser heating rates on the order of 109–1010 K/s by computational means, measurement of the kinetic energy distributions of desorbing aniline using a pump–probe method, and the determination of internal energies with resonance-enhanced multiphoton ionization spectroscopy. The measurements are compared to calculations of the surface temperature rise and the resulting desorption rates, based on a finite-difference mathematical description of pulsed laser heating. While the surface temperature of laser-heated silica reaches about 600–700 K at the time of desorption, the translational temperature of laser-desorbed aniline was measured to be Tkin=420±60 K, Tvib was 360±60 K, and Trot was 350±100 K. These results are discussed using different models for laser-induced thermal desorption from surfaces." @default.
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- W2006402753 date "1995-10-15" @default.
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- W2006402753 title "Laser-induced thermal desorption of aniline from silica surfaces" @default.
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- W2006402753 doi "https://doi.org/10.1063/1.470358" @default.
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