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- W2006522120 abstract "The reaction of C2 radicals with nitrogen was studied behind reflected shock waves by time dependent absorption and emission measurements. Mixtures of fullerene C60 highly diluted in argon were shock heated and used as C2 sources. Perturbation of the reaction system by addition of N2 results in changes of C2 absorption and causes strong CN emission. The C2 concentration was quantitatively monitored by ring dye laser absorption spectroscopy at ν = 19 355.60 cm-1. Simultaneously, the time behavior of spectrally resolved light emitted from the shock-heated mixtures was recorded by an intensified CCD camera in the wavelength range 315 nm ≤ λ ≤ 570 nm. By comparing the integrated C2 and CN emission signals for the Δv = 0 progressions, the CN concentration can be determined on the basis of the known C2 concentration and the relative line strengths. The experiments were performed in the temperature range 2896 K ≤ T ≤ 3420 K at pressures 1.68 bar ≤ p ≤ 2.03 bar. Evaluation of C2 and CN concentration measurements lead to the following rate coefficient for the reaction C2 + N2 ⇌ CN + CN: k3 1.5 × 1013 exp(−21 000 K/T) cm3 mol-1 s-1. The uncertainty in k3 is expected to be ±50%." @default.
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- W2006522120 date "1997-05-01" @default.
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- W2006522120 title "Perturbation Study on the Reaction of C<sub>2</sub> with N<sub>2</sub> in High-Temperature C<sub>60</sub>/Ar + N<sub>2</sub> Mixtures" @default.
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- W2006522120 doi "https://doi.org/10.1021/jp962779y" @default.
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