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• W2006818609 abstract "We present a detailed atomic-scale analysis of the postdeposition treatment of hydrogenated amorphous silicon (a-Si:H) thin films with H2 plasmas. The exposure of a-Si:H films to H atoms from a H2 plasma was studied through molecular-dynamics (MD) simulations of repeated impingement of H atoms with incident energies ranging from 0.04to5.0eV. Structural and chemical characterizations of the H-exposed a-Si:H films was carried out through a detailed analysis of the evolution of the films’ Si–Si pair correlation function, Si–Si–Si–Si dihedral angle distribution, structural order parameter, Si–H bond length distributions, as well as film surface composition. The structural evolution of the a-Si:H films upon exposure to H atoms showed that the films crystallize to form nanocrystalline silicon at temperatures over the range of 500–773K, i.e., much lower than those required for crystallization due to thermal annealing. The MD simulations revealed that during H exposure of a-Si:H the reactions that occur include surface H adsorption, surface H abstraction, etching of surface silicon hydrides, dangling-bond-mediated dissociation of surface hydrides, surface H sputtering/desorption, diffusion of H into the a-Si:H film, and insertion of H into strained Si–Si bonds." @default.
• W2006818609 created "2016-06-24" @default.
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• W2006818609 date "2006-09-01" @default.
• W2006818609 modified "2023-09-25" @default.
• W2006818609 title "Hydrogen-induced crystallization of amorphous silicon thin films. I. Simulation and analysis of film postgrowth treatment with H2 plasmas" @default.
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• W2006818609 doi "https://doi.org/10.1063/1.2229426" @default.
• W2006818609 hasPublicationYear "2006" @default.
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