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- W2007055176 abstract "Active sites are generated on sulfurated nickel surface by contacting with acetylene, on which the hydrogenation of acetylene and ethylene as well as the H2-D2 equilibration reaction proceed. These sites are wiped up by exhaustion of acetylene, and such reversible formation and vanishment of the active sites controls the partial hydrogenation of acetylene to ethylene on the sulfurated nickel catalyst. A nickel sulfide having an atomic ratio of SNi = 0.62 had the activity for the partial hydrogenation of acetylene, while a nickel sulfide of SNi = 0.96 had no catalytic activity. The surface composition of the sulfurated nickel estimated by Auger electron spectroscopy was a value of the ratio SNi = 0.69. From these results it is concluded that partial hydrogenation is enabled by reversible formation of active sites on sulfide with appropriate coordinative unsaturation of nickel atoms." @default.
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- W2007055176 date "1975-10-01" @default.
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- W2007055176 title "Catalysis and coordinative unsaturation of active sites on sulfurated nickel catalyst *1I. Reversible formation of active sites for partial hydrogenation of acetylene" @default.
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- W2007055176 doi "https://doi.org/10.1016/0021-9517(75)90231-6" @default.
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