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- W2007100460 abstract "The answer to the question in the title is “no” in the opinion of the authors. The decrease in the skeletal strain, rather than the slight differences in electronegativity between phosphorus and arsenic, seems to direct the As occupation of positions in the P framework. Ab initio calculations on [P7−xAsx]3⊖ systems with x = 0, 1, 2, 3, 7 show that the energy differences between the isomers contributes only ca. 10% of the activation energy for the valence tautomerism. Valence fluctuation therefore cannot favor any particular isomer." @default.
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- W2007100460 date "1991-07-01" @default.
- W2007100460 modified "2023-09-27" @default.
- W2007100460 title "Do Partial Charges Alone Govern the Relative Stability of the Isomeric Heptaheteronortricyclane Anions[P7−xASx]3⊖?" @default.
- W2007100460 doi "https://doi.org/10.1002/anie.199108281" @default.
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