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- W2007154706 abstract "Optical side bands are observed in the spectrum of TmAsO4. Measurements of their polarisation and intensity are made as a function of magnetic field. These results are interpreted using a tight binding theory developed earlier. It is found that the most intense side band is caused by off-diagonal exchange (Γ3 − Γ1 and Γ4 − Γ1) between the ground doublet and the excited singlet arising from virtual phonon exchange. The less intense side bands are caused by a large number of exchange interactions and the analysis is less clear.Es wurden die Polarisation und die Magnetfeldabhangigkeit der Intensitat von Nebenlinien im Absorptionsspektrum von TmAsO4 untersucht. Die gewonnenen Ergebnisse werden mit Hilfe eines „tight-binding”-Modells interpretiert. Die intensivste Nebenlinie wird durch einen virtuellen Phononaustausch zwischen dem Grundzustandsdublett und einem angeregten Singulett ver-ursacht. Bei anderen Nebenlinien, die durch eine Vielzahl von Austauschwechselwirkungen induziert werden, fuhrte die Analyse der Wechselwirkungen nicht zu einer eindeutigen Zuordnung." @default.
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- W2007154706 date "1977-05-01" @default.
- W2007154706 modified "2023-09-24" @default.
- W2007154706 title "Optical Side Bands in a Cooperative Jahn-Teller Material: TmAsO4" @default.
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- W2007154706 doi "https://doi.org/10.1002/pssb.2220810116" @default.
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