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- W2007174915 abstract "Studies have been carried out on (U,Ce)O2−x to assist the understanding of oxygen behaviour in the fast reactor fuel (U, Pu)O2−x. Oxygen potentials at 1123 K and lattice parameters after rapid cooling to room temperature have been determined as functions of O/M ratio for Ce/(U + Ce) ratios of 0.148 and 0.282. The results show some similarities between the two mixed oxides, but also important differences. The Markin-McIver rule, that oxygen potential at a given temperature is a function only of the supposed plutonium valence, does not apply with cerium. Simple cluster models are basically inconsistent with experimental data and a complex cluster model requires further development before it can account for the oxygen potential behaviour of (U, Ce)O2−x. The ratio of lattice parameter change to O/M ratio change in U1−yCeyO2−x is not strongly dependent on y and averages 0.30 Å, slightly greater than the corresponding value for U1−yPuyO2−x. A transition to a room-temperature two-phase structure occurs at an O/M ratio of about 1.985 for y = 0.282." @default.
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- W2007174915 date "1983-06-01" @default.
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- W2007174915 title "Oxygen potential and lattice parameter measurements in (U, Ce)O2 − zx" @default.
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- W2007174915 doi "https://doi.org/10.1016/0022-3115(83)90101-0" @default.
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